The data analysis reveals multiple episodes of smoke intrusions into the stratosphere through both pyroconvection (PyroCb) and synoptic-scale process (warm conveyor belt, WCB). Model simulations using MOCAGE chemistry-transport model, constrained by emission data from GFAS (Global Fire Assimilation System) are shown to accurately capture the synoptic-scale WCB-driven uplift of smoke from the lower/middle troposphere to the lowermost stratosphere and reproduce the spatial evolution of the aerosol plumes. The MOCAGE simulation is validated against the multiwavelength LILAS lidar observations in Northern France.
We show that despite the exceptional vigor of the 2023 Canadian wildfires, the depth of their stratospheric impact was surprisingly shallow and limited to the lowermost stratosphere. Conversely, the long succession of moderate-strength PyroCb events, combined with numerous episodes of smoke uplift across the tropopause by WCB process, led to unparalleled levels of pollution at the commercial aircraft cruising altitudes throughout the season.
The research was supported by the French Agence Nationale de la Recherche (ANR) PyroStrat project (Grant No: 21-CE01-0028-01)
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