To better understand the structural aspects of the intensification process, a Lagrangian perspective is explored herein of the localized stirring around VHTs and their vortical remnants, as well as the evolution and stirring of $\theta_e$. Recently developed finite-time Lagrangian methods can locate time-dependent structures effectively, but are designed for two-dimensional flows with weak time-dependence rather than the highly time-dependent, three-dimensional, turbulence associated with the VHTs. In this paper, we summarize new Lagrangian techniques that have been developed for three-dimensional velocity fields and we apply these techniques to study VHT and $\theta_e$ phenomenology. Our primary findings are that VHTs are coherent Lagrangian vortices that create a turbulent mixing environment; and associated with VHTs are hyperbolic structures that modulate the aggregation of VHTs and their vortical remnants. Although the azimuthally-averaged inflow is responsible for the inward advection of boundary layer $\theta_e$, the Lagrangian coherent structures modulate the boundary layer convection by stirring $\theta_e$ along organized attracting boundaries. We identify additional coherent structures above the boundary layer, which are responsible for organizing the remnants of the convective vortices. These hyperbolic structures form initially as boundaries between VHTs, but they outlive the VHTs and eventually form the primary eyewall as the vortex attains maturity.