In this study we used CLM4.5 (Community Land Model version 4.5) as the land-surface model. Meteorological data from a high-resolution WRF (Weather Research and Forecasting Model) simulation for the summer of 2012 were used to drive CLM4.5 and also a transport model (STILT; Stochastic Time-Inverted Lagrangian Transport Model). WRF-STILT was used to model the footprints of atmospheric CO2 observations at three sites in the Regional Atmospheric Continuous CO2 Network in the Rocky Mountains (Rocky RACCOON) (Hidden Peak, Niwot Ridge, and Storm Peak Laboratory). The footprints were combined with the modeled surface fluxes from CLM4.5 in order to simulate CO2 concentrations at each site. Surface CO2 emissions associated with anthropogenic emissions and wildfires (both minor components in comparison with the biospheric fluxes in the study region) were taken from EDGAR (Emission Database for Global Atmospheric Research) and WFEI (Wildland Fire Emission Inventory) inventories, respectively. Modeled CO2 concentrations were then compared against observations at each site, and the differences were used to guide parameter adjustments in CLM4.5. The initial results of this modeling effort will be presented.