Scalar spectra and cospectra from the ASL show that large-scale motions that scale on outer-layer parameters do interact with active motions that scale on inner-layer parameters. It is proposed that this is so because outer-layer motions control the areal pattern of surface wind velocities, and because coherent structures are triggered where strong local convergence of the surface wind intensifies local shear stress. The locations and sizes of coherent turbulent structures, which carry most of the flux, are thereby controlled by outer-layer motions. This case is supported by drawing on results from wall-bounded shear flows in both the ASL and the laboratory. Such flows have many similarities despite great differences in Reynolds numbers and roughness of the walls. We conclude that transport processes in the ASL depend on the outer-layer scales, that Townsends hypothesis fails and therefore that Monin-Obukhov similarity theory is flawed.