- Ni increases as the cooling rate of air parcel (–dT/dt) increases,
- Ni decreases as initial water vapor mixing ratio (X0) increases,
- Ni decreases as accommodation coefficient (αd) increases, and
- Ni decreases as radius of aerosol particles (r) increases, especially when r is greater than ~0.5 μm.
The fourth feature above is explained by the improved water uptake efficiency by aerosols with large nuclei (thus large ice particles) and suppression of new ice particle formation (hereafter referred to as “effect 1”). Another effect, that is, the increase of ice nucleation rate due to the increase of aerosol volume (hereafter referred to as “effect 2”), need to be considered. Due to this effect2, larger aerosols could nucleate under lower RHi condition.
The present paper discusses the behavior of Ni under the existence of bimodal aerosol distribution paying special attention to these two contrasting effects. The experimental condition is set to –dT/dt = 2.8 K h−1, X0= 6 ppmv, and αd =0.3, that lead to Ni = 104 L−1 for monodisperse aerosol radius of 0.05 μm. In order to focus on the interaction between bimodal aerosols with different radius (ra, rb), the number concentrations of two aerosol types are set to the same (105 L-1). As the first step of our analysis, we fix ra = 0.05 μm and sweep rb from 0.01 to 10 μm, and discuss about the result by focusing on Ni and number concentrations of ice nucleated from two size of aerosols (Nia, Nib).
It is readily seen that Nia decreases as rb increases because of the effect 2. On the other hand, Nib takes maximum at rb = 0.084 μm. When rb is much smaller than ra, aerosols with radius ra nucleate at lower RHi, suppressing the nucleation of aerosols with radius rb. On the other hand, when rb is larger than ra, the proportion of Nib in Ni becomes larger due to effect 2. However, when rb is larger than 0.084 μm, the suppression of Nib by effect 1 along with increase of rb exceeds the promotion of Nib by effect2. Another point of special interest is that Ni takes maximum at rb = 0.035 μm exceeding that at ra = rb = 0.05 μm. This may be the result of effect2 of the aerosols rb leading to the decrease in Nia and increase in Nib. The results from the case of different ra will be also discussed at the time of presentation.
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