It is found that the land surface temperature underneath the aerosol layer is sensitive to the aerosol vertical distribution: the lifted layer of aerosols results in a significant cooling of the underlying land surface, while the PBL profile makes very little cooling.
The mechanism of the aerosol effect on precipitation distribution is investigated by examining the correspondence between aerosol heating profile, changes of precipitation and the atmospheric convective instability. The direct aerosol heating of the near-surface air increases the Convective Available Potential Energy (CAPE) whereas the heating above the boundary layer decreases CAPE. Meanwhile, the regionally concentrated low-level aerosol heating tends to cause large-scale rising motion over time, which increases CAPE by decreasing the mid-level temperature. The net CAPE change is small for the lifted profile (i.e., profile elevated above PBL) because the CAPE increase by the mid-level cooling is counteracted by the CAPE decrease through the direct haze heating above the PBL. The precipitation increase averaged over the aerosol area is much larger when the PBL profile is used than when the lifted profile is used in the CCM3 with a CAPE-based convective parameterization closure. The sensitivity of the aerosol effect to convective parameterization closure is tested using a new closure, which is based on the environmental contribution to CAPE (CAPEe). It is shown that when this closure is used in CCM3, the precipitation increase averaged over the aerosol area is small regardless of the vertical profile. This is because the direct heating of either profile decreases CAPEe opposing the CAPEe increase by the mid-level cooling.
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